Rather than what I do not like, how about what I like:
1) Videos that are about 15 minutes.
2) Being able to download the text of the video
3) Being able to download the power points
4) Pertinent exercises - with an optional video to show one solution
5) Good volume control - on first video I set my volume and I do not need to change it for each video - I know sounds trivial
6) Being able to skip back 15 seconds
7) I really like it when they have a 'Explore more' page with links to learn more indepth on the topic.
8) If it is a 'Read', then I prefer a PDF that is ideally even number of pages (to print both sides)
9) If it is a 'Read', then font size 12
10) All material that I might print, be organized with the idea that I would print it - no DOS windows of all black that will chew up all my ink
11) Nice feature would be a questions section
12) Easy to, at a glance, see where you left off the last time