Some of it might benefit AVR, which being 8-bit, shares some of the same problem space. But most of the changes we've made so far are of the kind where LLVM says "this doesn't happen", or "when it does, it's not important." And now the 6502 says, "uh, I actually do need that..."
So in absolute terms of maximizing the flexibility of LLVM, yes, the changes do seem to be broadly useful, but they're mostly in a direction that doesn't benefit most processors all that much.
For example, the 6502 really wants to replace stack usage with global usage; we do this absolutely whenever possible. Other targets actually run the opposite transformation; they replace global variables with stack ones! Placing things on the stack maximizes the chance it'll be in a fast CPU cache (or that it may be folded into a register; this does apply to us too.)