For the display, this poster has something similar and talks about a datasheet - there's even a pinout for the flex cable (and it's supposedly SPI) [0]. It's for the 2.6" version not the 2.7 though so might be totally different. A comment on the post (by this person [1]) claims that they have working cleanroom CC2510 code that drives the display but who knows.
Great project anyway - I look forward to part two (and what you find on that flash chip)!
(Edit: sorry if you know this already, but there's a manual for the labels themselves [2] implying the setup page is permanently stored in one of the 4 slots - hopefully in that external flash chip)
0: https://epongenoir.blogspot.com/2017/10/
1: http://andreiprojects.blogspot.com/
2: https://fccid.io/2ACQM-EDG1-0260-A/User-Manual/User-Manual-5...